This book focuses on the development of high-performance carbon electrodes for sodium ion batteries (SIBs). By proposing folded-graphene as the high-density cathode with excellent rate capability, it provides insight into the interplay between oxygen functional groups and folded texture. It also highlights the superiority of ether electrolytes matching with carbon anodes, which are shown to deliver largely improved electrochemical performance. The achievements presented offer a valuable contribution to the carbon-based electrodes in SIBs.
Erscheinungsdatum: 02.11.2023

lgli/1847.pdf

lgrsnf/1847.pdf

Singapore, Singapore

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Supervisor’s Foreword
Abstract
Acknowledgements
Contents
Abbreviations
1 Introduction
1.1 Overview
1.2 Recent Progress of SIBs in Academy and Industry
1.3 Potential Application of Carbon Materials as Cathode
1.4 Practical Carbon Anodes Towards High Energy or Power Density
1.5 The Main Research Topics and Content
References
2 Experimental Details
2.1 Main Reagents and Raw Materials
2.2 Main Equipment
2.3 Characterization
2.3.1 Structural Characterization
2.3.2 Electrochemistry
3 Folded-Graphene as an Ultrafast Cathode Material
3.1 Introduction
3.2 Experimental Section
3.3 High-Density Folded-Graphene Cathode for SIBs
3.4 Ultrafast High-Volumetric Sodium Storage via Folded-Graphene Cathode
3.5 Summary
References
4 The Interplay of Oxygen Functional Groups and Folded Texture in Folded-Graphene Cathode
4.1 Introduction
4.2 Experimental Section
4.3 The Critical Roles of Oxygen Functional Groups and Folded Texture
4.4 The Interplay of Oxygen Functional Groups and Folded Texture
4.5 Summary
References
5 Achieving Efficient Sodium Storage on Carbon Anodes with Ether-Derived Solid Electrolyte Interphase (SEI)
5.1 Introduction
5.2 Experimental Section
5.3 Achieving Efficient Sodium Storage on Diverse Carbon Anodes with Ether-Based Electrolytes
5.4 Advantages of Ether-Derived SEI
5.5 Summary
References
6 Evolution of the Electrochemical Interface with Ether-Based Electrolytes
6.1 Introduction
6.2 Experimental Section
6.3 Improved Sodiation Depth in Ether-Based Electrolytes
6.4 Evolution of Interfacial Electrochemistry with Ether-Based Electrolytes
6.5 Summary
References
7 Conclusion and Perspective
7.1 Conclusion
7.2 Perspective
References
Personal Statement
Resume and Research Achievements
Resume
Publications
Awards
Conference Contribution

2024-03-20